| 角色 | 饰演者 | 角色介绍 |
| Clumsy (voice) | 安东·尤金 | |
| Smurfette (voice) | 凯蒂·派瑞 | |
| Gargamel | 汉克·阿扎利亚 | |
| Papa (voice) | 乔纳森·温特斯 | |
| Gutsy (voice) | 艾伦·卡明 | |
| Brainy (voice) | 弗莱德·阿米森 | |
| Grouchy (voice) | 乔治·洛佩兹 | |
| Greedy (voice) | 基南·汤普森 | |
| Handy (voice) | 杰夫·福克斯沃西 | |
| Patrick Winslow | 尼尔·帕特里克·哈里斯  | |
| Grace Winslow | 杰玛·梅斯 | |
| Odile | 索菲娅·维加拉 | |
| Henri | 蒂姆·古恩 | |
| Model | Madison McKinley | |
| Model | Meg Phillips | |
| Newscaster | Julie Chang | |
| Newscaster | Roger Clark | |
| Bluetooth Businessman | Mark Doherty | |
| Young Woman | Minglie Chen | |
| Guy in Plaid Shirt | Sean Kenin | |
| Bum | Victor Pagan | |
| Cabbie | Mahadeo Shivraj | |
| Anjelou Employee | Adria Baratta | |
| Odile's Mother | Paula Pizzi | |
| Waiter | Andrew Sellon | |
| Little Sister | Julianna Rigoglioso | |
| Blonde Sister | Daria Rae Figlo | |
| Toy Salesperson | Bradley Gosnell | |
| Toy Store Parent | Heidi Armbruster | |
| Toy Store Parent | Finnerty Steeves | |
| Parent with Girls | John Speredakos | |
| Kicking Girl | Skai Jackson | |
| Skateboard Kid | Alex Hall | |
| Skateboard Kid | Eric Redgate | |
| FAO Custodian | Jojo Gonzalez | |
| Cop | Scott Dillin | |
| Cop (as Tyree M. Simpson) | Tyree Michael Simpson | |
| Inmate Bubba | Sean Reinggold | |
| Bubba's Inmate Friend | Mario D'Leon |
